Measurement of the differential and total cross-sections ofγ-ray emission induced by 14.1 MeV neutrons for C, Al, Si, Ca, Ti, Cr, and Fe using the tagged neutron method

  • In this work, differential cross sections of $ \gamma $-ray emission produced in nuclear reactions induced by 14.1 MeV neutrons are measured for the 4.439 MeV line from carbon, as well as for 10 individual $ \gamma $-ray lines from aluminum, 6 from silicon, 8 from calcium, 16 from titanium, 6 from chromium, and 14 from iron. The measurements were conducted using the tagged neutron method with four LaBr 3(Ce) scintillation detectors positioned at angles of 25°, 45°, 60°, and 70° relative to the generator target – sample center axis. A neutron generator that can produce 16 separate beams of tagged neutrons was employed, which combined with the detector system, enabled the determination of differential cross-sections for 64 distinct angle values in the range of 17° to 89°. To simplify data visualization, the angular distributions were divided into 5° intervals, with weighted mean values of the angle and differential cross-section calculated for each interval. Corrections for multiple neutron scattering and attenuation, $ \gamma $-ray attenuation, and total detection efficiency computed using GEANT4 were accounted for in the cross-section calculations. Additional measurements were performed to validate the correction calculations. The total $ \gamma $-ray emission cross-sections were obtained by approximating the angular distributions with even-order Legendre polynomial expansions up to the 6th degree, followed by integration over the full solid angle. The total systematic error for the obtained data was estimated as 9.1%.
  • 加载中
  • [1] Karolina Kolos, Vladimir Sobes, Ramona Vogtet al., Phys. Rev. Research4, 021001 (2022) doi:10.1103/PhysRevResearch.4.021001
    [2] I. Ruskov, Yu. Kopatch, V. Bystritskyet al., EPJ Web Conf.146, 03024 (2017) doi:10.1051/epjconf/201714603024
    [3] I. Ruskov, Yu. Kopach, V. Bystritskyet al., EPJ Web Conf.256, 00014 (2021) doi:10.1051/epjconf/202125600014
    [4] V. Valkovic, in14 MeV Neutrons: Physics and Application, Vol. 2, edited by Vladivoj Valkovic (Boca Raton: CRC Press, 2016), p. 17
    [5] V. Valkovic, in14 MeV Neutrons: Physics and Application, Vol. 7, edited by Vladivoj Valkovic (Boca Raton: CRC Press, 2016), p. 256
    [6] I. Bolshakov, M. Kolesnik, M. Sorokinet al., Int. J. Miner. Process. Extr. Metall.5(4), 54 (2020) doi:10.11648/j.ijmpem.20200504.11
    [7] V. Y. Alexakhin, A. I. Akhunova, E. A. Razinkovet al., Phys. Atom. Nuclei85, 1866 (2022) doi:10.1134/S1063778822100039
    [8] S. Bishnoi, T. Patel, R. G. Thomaset al., Eur. Phys. J. Plus135, 428 (2020) doi:10.1140/epjp/s13360-020-00402-y
    [9] D. N. Grozdanov, N. A. Fedorov, V. M. Bystritskiet al., Phys. Atom. Nuclei81, 588 (2018) doi:10.1134/S106377881805006X
    [10] N. A. Fedorov, T. Y. Tretyakova, V. M. Bystritskyet al., Phys. Atom. Nuclei82, 343 (2019) doi:10.1134/S1063778819040094
    [11] N. A. Fedorov, D. N. Grozdanov, Y. N. Kopatchet al., Eur. Phys. J. A57, 194 (2021) doi:10.1140/epja/s10050-021-00503-x
    [12] I. D. Dashkov, N. A. Fedorov, D. N. Grozdanovet al., Bull. Russ. Acad. Sci. Phys.86, 893 (2022) doi:10.3103/S1062873822080056
    [13] Y. N. Kopach and M. G. Sapozhnikov, Phys. Part. Nuclei55, 55 (2024) doi:10.1134/S106377962401009X
    [14] Y. N. Kopatch, D. N. Grozdanov, N. A. Fedorovet al., Phys. Part. Nuclei Lett.22, 276 (2025) doi:10.1134/S154747712470225X
    [15] V. E. Scherrer, R. B. Theus, and W. R. Faust, Phys. Rev.91, 1476 (1953) doi:10.1103/PhysRev.91.1476
    [16] J. Benveniste, A. C. Mitchell, C. D. Schraderet al., Nucl. Phys.19, 448 (1960) doi:10.1016/0029-5582(60)90255-8
    [17] D. T. Stewart and P. W. Martin, Nucl. Phys.60(2), 349 (1964) doi:10.1016/0029-5582(64)90669-8
    [18] I. L. Morgan, J. B. Ashe, D. O. Nellis, Div. of Tech. Info. U.S. AEC Reports, No. 22012, (Texas Nuclear Corp., Austin, TX, USA, 1964), p.158; EXFOR data: https://www-nds.iaea.org/EXFOR/12695
    [19] F. C. Engesser and W. E. Thompson, J. Nucl. Energy21(6), 487 (1967) doi:10.1016/0022-3107(67)90020-2
    [20] G. Clayeux, G. Grenier, Saclay Reports, No.3807, (Centre d'Etudes de Limeil, Villeneuve-Saint-Georges, France, Centre d`Etudes Nucleaires, 1969)
    [21] T.C. Martin, G.H. Williams, Oak Ridge Operations Office, contract report, No. 2791-32, (Texas Nuclear Corp., Austin, TX, USA, 1971), p.7
    [22] D. Spaargaren and C. C. Jonker, Nucl. Phys. A161(2), 354 (1971) doi:10.1016/0375-9474(71)90374-5
    [23] V. C. Rogers, V. J. Orphan, C. G. Hootet al., Nucl. Sci. Eng.58(3), 298 (1975) doi:10.13182/NSE75-A26779
    [24] V. M. Bezotosnyi, V. M. Gorbachev, L. M. Suvorovet al., Yad. Konst.19, 7 (1975)
    [25] S. Zong-Renet al., Chin. J. Nucl. Phys.1, 45 (1979)
    [26] Y. Hino, S. Itagaki, T. Yamamotoet al., Dept. of Nucl. Engineering Reports, No. 34, (Tohoku Univ., Sendai, Japan, 1979)
    [27] I. Murata, J. Yamamoto, A. Takahashi,Differential cross sections for gamma-ray production by 14 MeV neutrons with several elements in structural materials, inProceedings of the International Conference on Nuclear Data for Science and Technology held at Mito, Japan, May 30-June 3, edited by S.Igarasi, (Japan: Japan Atomic Energy Research Institute, 1988), p. 275 https://wwwndc.jaea.go.jp/nd1988/
    [28] H. Zhou,Y. Yan, Tanglin, Wen Shenlinet al., Chin. J. Nucl. Phys.11(2), 63 (1989)
    [29] K. Hasegawa, M. Mizumoto, S. Chibaet al., Gamma-ray production cross section measurements of some structural materials between 7.8 and 13.0 MeV, inProceedings of the International Conference on Nuclear Data for Science and Technology, held at the Forschungszentrum Julich, Fed. Rep. of Germany, 13−17 May 1991, edited by Syed M. Qaim, (Germany: Springer-Verlag Berlin Heidelberg, 1992), p. 329 https://doi.org/10.1007/978-3-642-58113-7
    [30] A. I. Lashuk and I. P. Sadokhin, Vop. At. Nauki i Tekhn., Ser.Yaderno-Reak. Konstanty1, 26 (1994)
    [31] I. M. Kadenko, V. A. Plujko, B. M. Bondaret al., Yaderna Fizika ta Energetika17, 349 (2016)
    [32] A. M. McEvoy, H. W. Herrmann, Y. Kimet al., Phys. Rev. C103, 064607 (2021) doi:10.1103/PhysRevC.103.064607
    [33] K. J. Kelly, M. Devlin, J. M. O'Donnellet al., Phys. Rev. C104, 064614 (2021) doi:10.1103/PhysRevC.104.064614
    [34] K. J. Kelly, M. Devlin, J. M. O'Donnellet al., Phys. Rev. C108, 014603 (2023) doi:10.1103/PhysRevC.108.014603
    [35] J. M. Gordon, B. L. Goldblum, J. A. Brownet al., Phys. Rev. C111, 044608 (2025) doi:10.1103/PhysRevC.111.044608
    [36] J. K. Dickens, G. L. Morgan, G. T. Chapmanet al., Nucl. Sci. Engineering62, 515 (1977) doi:10.13182/NSE77-A26989
    [37] D. N. Grozdanov, Prusachenko, P. S., Fedorovet al., Eur. Phys. J. A61, 224 (2025) doi:10.1140/epja/s10050-025-01703-5
    [38] E. M. Burymov, Sov. J. Nucl. Phys.9, 546 (1969)
    [39] V. N. Bochkarev and V. V. Nefedov, Sov. J. Nucl. Phys.1, 574 (1965)
    [40] A. Pavlik, H. Hitzenberger-Schauer, H. Vonachet al., Phys. Rev. C57, 2416 (1998) doi:10.1103/PhysRevC.57.2416
    [41] S. Hlavac, M. Benovic, E. Betaket al.,Cross Sections for Discrete \begin{document}$\gamma$\end{document} Ray Production in Interactions of 14.6 MeV Neutrons with Light and Medium Heavy Nuclei, IAEA Nucl. Data Section report to the I.N.D.C., Rep. No. 412, p.12 (1999), (IAEA, Vienna, Austria, 1999) http://www-nds.iaea.org/publications/indc/indc-nds-0412/
    [42] V. C. Rogers, V. J. Orphan, C. G. Hootet al.,Spectral gamma-ray production cross-section measurements from threshold to 20 MeV, inProceedings of the Conference on Nuclear Cross Sections and Technology, Washington, USA, 1975, edited by Roald A. Schrack, Charles D. Bowman, (USA: Department of Commerce, National Bureau of Standards, Institute for Basic Standards, Center for Radiation Research, 1975), Vol. 2, p. 766 https://nvlpubs.nist.gov/nistpubs/Legacy/SP/nbsspecialpublication425v2.pdf
    [43] H. Zhou and G. Huang, Nucl. Sci. Eng.125(1), 61 (1997) doi:10.13182/NSE97-A242545
    [44] K. Nyberg-Ponnert, B. Jonsson, and I. Bergqvist, Phys. Scr.4, 165 (1971) doi:10.1088/0031-8949/4/4-5/004
    [45] Z. Hongyu, T. Lin, Y. Yiminget al.,Gamma ray production cross sections for the interactions of 14.9 MeV neutrons with C, Al, V, Fe and Nb at 90 degrees, Chinese report to the I.N.D.C., Rep. No INDC(CPR)-010/L, (IAEA NDC, Vienna, Austria, 1986) https://www-nds.iaea.org/publications/indc/indccpr010L.pdf.
    [46] J. T. Prud'homme, I. L. Morgan, J. H. MC. Craryet al., A study of neutrons and gamma rays from neutron induced reactions in several elements, Air Force Spec. Weap. Center Kirtland A.F.B. Repts., Rep. No 60-30, (Texas Nuclear Corp., Austin, Texas, USA, 1960).
    [47] P. W. Martin and D. T. Stewart, J. Nucl. Energy19(6), 447 (1965) doi:10.1016/0368-3230(65)90053-4
    [48] U. Abbondanno, R. Giacomich, M. Lagonegroet al., J. Nucl. Energy27(4), 4 (1973) doi:10.1016/0022-3107(73)90058-0
    [49] G. Grenier, B. Duchemin, and D. Parisot,Differential gamma-ray production cross sections measured in Si \begin{document}$(n, X\gamma)$\end{document} , Cr \begin{document}$(n, X\gamma)$\end{document} and Ni \begin{document}$(n, X\gamma)$\end{document} reactions for incident neutrons between 3 and 7 MeV and also at 14.1 MeV(in French), Report from CEC-Countries and CEC to NEANDC, Rep. No. 161U, (CEA/DAM Ile-de-France, Bruyeres-le-Chatel, Arpajon, France, 1974) https://inis.iaea.org/records/jwywe-zwf06
    [50] K. A. Connell and A. J. Cox, Int. J. Appl. Radiat. Isot.26(2), 71 (1975) doi:10.1016/0020-708X(75)90105-2
    [51] D. M. Drake, E. D. Arthur, and M. G. Silbert, Nucl. Sci. Eng.65(1), 1 (1978) doi:10.13182/NSE78-A27125
    [52] V. M. Bezotosnyj, V. M. Gorbachjov, M. S. Shvetsovet al.,The spectra and formation cross-sections of the discrete gamma-lines in the nonelastic interaction of 14 MeV neutrons with Mg, Si, P, S, Ti and Zn nuclei(In Russian), USSR report to the I.N.D.C., Rep. No. INDC(CCP)-169_VOL_IV, (IAEA NDS, Vienna, Austria, 1980), p.21https://www-nds.iaea.org/publications/indc/indc-ccp-0169_vol_II.pdf
    [53] G. Fan, H. Zhou, X. Zhuet al.,Progress in the Measurement of Gamma-Ray Production Cross Sections Induced by 14.9 MeV Neutrons, In: Qaim, S.M. (eds) InProceedings of the International Conference on Nuclear Data for Science and Technology held at the Forschungszentrum Jülich, Fed. Rep. of Germany, 13-17 MaY 1991, edited by Syed M. Qaim, (Germany: Springer-Verlag Berlin Heidelberg, 1992), p. 332 https://doi.org/10.1007/978-3-642-58113-7_95
    [54] M. Drosg, R. C. Haight, and D. M. Drake,Double-differential gamma-ray production: cross sections and spectra of Al, Si and Fe for 8.51, 10.00, 12.24 and 14.24 MeV neutrons, Los Alamos Scientific Lab., Rep. No. 02-16, (Los Alamos National Laboratory, New Mexico, USA, 2002)
    [55] H.-Y. Zhou, F.-G. Deng, W. Chenget al., Nucl. Instrum. Methods Phys. Res. A648(1), 192 (2011) doi:10.1016/j.nima.2011.04.014
    [56] A. Negret, C. Borcea, D. Bucurescuet al., Phys. Rev. C88, 034604 (2013) doi:10.1103/PhysRevC.88.034604
    [57] M. Boromiza, C. Borcea, P. Dessagneet al., Phys. Rev. C101, 024604 (2020) doi:10.1103/PhysRevC.101.024604
    [58] A. P. Arya, D. L. Campbell, and R. D. Wilson, Bull. Am. Phys. Soc.12, HD4 (1967)
    [59] W. Breunlich, G. Stengl, and H. Vonach, Z. Naturforsch. A26, 451 (1971) doi:10.1515/zna-1971-0315
    [60] G. L. Morgan and D. C. Larson,The Ti \begin{document}$(n, x\gamma)$\end{document} reaction cross section for incident neutron energies between 0.3 and 20.0 MeV, Oak Ridge National Lab. technical memo, No.6323, (Oak Ridge National Laboratory, Oak Ridge, TN, USA, 1978) https://inis.iaea.org/records/806kn-26t18
Baidu
map